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Trigonally distorted octahedron and phase coupling: Cr(acac)_3

This is a single-point calculation without optimization. By the aid of two geometric parameters, a trigonally distorted octahedron is defined: theta+ controls compression, phi torsion along the trigonal axis. In the CON block, chelate connectivity as well as phase coupling parameters are specified (see section 3.2.6). The line `3 D3 14' defines: 3 electrons, trigonal symmetry, printout of the first 14 states (resp. 7 Kramers doublets since it is a calculation with spin-orbit coupling on a system with odd electron number).

Cr(acac)3
Lit: Atanasov, Schoenherr, IC 29,4545 (1990), Fig. 4

3 D3 14

VAR
*
10Dq        = 18700
epis        =  1000
epis'       =     0
pic/2pis0   =     0.6
B           =   500
C           =  3400
zeta        =   245
theta+   =    53.8
phi      =    60.8
epis0    = epis / 2 + epis' / 2
epic     = 2 * epis0 * pic/2pis0
episdiff = epis - epis'
esig     = 10Dq / 3 + 2 * epis0 / 3 + 2 * epic / 3 
theta-   = 180 - theta+
phi1     = phi  /   2
phi2     = phi1 + 120
phi3     = phi1 + 240
phi4     = phi  /  -2
phi5     = phi4 + 120
phi6     = phi4 + 240

AOM
esig epis0 epic
esig epis0 epic
esig epis0 epic
esig epis0 epic
esig epis0 epic
esig epis0 epic

TPP
theta+ phi1
theta+ phi2
theta+ phi3
theta- phi4
theta- phi5
theta- phi6

CON
1 4 episdiff episdiff
2 5 episdiff episdiff
3 6 episdiff episdiff

VEE 0 B C

HSO zeta

RUN



Heribert Adamsky
Sat Sep 14 16:23:16 MET DST 1996